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Enhanced Removal Efficiency of Malachite Green Dye Using Gambir Leaf Extract-Modified NiFe LDH Composites: A Study of Cationic Dye Adsorption

Bulletin of Chemical Reaction Engineering & Catalysis · Vol. ume (2024) · hlm. 573–584

DOI
10.9767/bcrec.20215
ISSN
1978-2993
Terbit
2024-12-30
Penerbit
Masyarakat Katalis Indonesia - Indonesian Catalyst Society (MKICS)
Bahasa
eng
Lisensi
creativecommons.org/licenses/by-sa/4.0

Abstrak

A NiFe layered double hydroxide (LDH) composite with Uncaria gambir (UG) leaf extract was successfully synthesized. The composite (NiFe-UG LDH) and the base material (NiFe LDH) were identified using X-ray Diffraction (XRD), Fourier Transform Infra Red (FTIR), and Brunauer-Emmett-Teller (BET) Surface Area techniques. The XRD and FTIR results revealed the incorporation of gambier leaf extract into the NiFe LDH structure, as indicated by the combined diffraction patterns and spectral features. The BET analysis indicated a decrease in the surface area of NiFe-UG LDH compared to that of NiFe LDH, suggesting that active compounds from the gambier leaf extract effectively coated the LDH surface and blocked its pores. During malachite green (MG) adsorption, NiFe-UG demonstrated faster adsorption kinetics and a higher adsorption efficiency, reaching 96.420% compared to 92.085% for NiFe LDH. While both materials followed pseudo-first-order kinetics, their isotherm behaviors differed: NiFe-UG adhered to the Langmuir model, indicating monolayer adsorption, whereas NiFe LDH followed the Freundlich model, signifying multilayer adsorption. Further analysis suggested that adsorption in NiFe LDH was primarily governed by physisorption, while in NiFe-UG, a combined physisorption-chemisorption mechanism occurred. These results underscore the enhanced adsorption capacity of the composite material, attributed to the introduction of additional functional groups from the gambier leaf extract. Copyright © 2024 by Authors, Published by BCREC Publishing Group. This is an open access article under the CC BY-SA License (https://creativecommons.org/licenses/by-sa/4.0).

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  • Sriwijaya University
  • Universitas Palembang
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Rekan penulisOrganisasiArtikel bersama
Risfidian MohadiSriwijaya University16
Neza Rahayu PalapaSriwijaya University10
Alfan WijayaSriwijaya University8
Nur AhmadSriwijaya University7
Tarmizi TaherSriwijaya University7
Mardiyanto MardiyantoSriwijaya University7
Amri AmriSriwijaya University6
Nova YuliasariSriwijaya University4
Patimah Mega Syah Bahar Nur SiregarSriwijaya University4
Yulizah HanifahSriwijaya University4
Muhammad SaidSriwijaya University4
Idha RoyaniSriwijaya University3
Novie JuleantiSriwijaya University3
Sahrul WibiyanSriwijaya University2
Arini Fousty BadriSriwijaya University2
Fitri Suryani ArsyadSriwijaya University2
Normah NormahSriwijaya University2
NormahSriwijaya University2
Eliza ElizaSriwijaya University2
Muhammad SaidSriwijaya University2
Haris KriswantoroUniversitas Palembang1
Benyamin LakitanSriwijaya University1
Andi WijayaSriwijaya University1
Elfita ElfitaSriwijaya University1
Zaqiya Artha ZaharaSriwijaya University1
Rohmatullaili RohmatullailiSriwijaya University1
Laila HanumSriwijaya University1
Elda MelwitaSriwijaya University1
Suheryanto SuheryantoSriwijaya University1
Addy RachmatSriwijaya University1
Bakri Rio RahayuSriwijaya University1
Nurlisa HidayatiSriwijaya University1
Mikha Meilinda ChristinaSriwijaya University1
Ferlinahayati FerlinahayatiSriwijaya University1
Muhammad BadaruddinSriwijaya University1
MardiyantoAfiliasi tidak diketahui1
AmriAfiliasi tidak diketahui1

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Sumber metadata: OAI-PMH (metadata jurnal) https://journal.bcrec.id/index.php/bcrec/oai, pertama di-harvest 8 Nov 2026, terakhir terlihat 8 Nov 2026.
Metadata asli (oai_dc) 
<oai_dc:dc xmlns="http://www.openarchives.org/OAI/2.0/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:oai_dc="http://www.openarchives.org/OAI/2.0/oai_dc/" xmlns:xsi="http://www.w3.org/2001/XMLSchema-instance" xsi:schemaLocation="http://www.openarchives.org/OAI/2.0/oai_dc/  http://www.openarchives.org/OAI/2.0/oai_dc.xsd">
	<dc:title xml:lang="en-US">Enhanced Removal Efficiency of Malachite Green Dye Using Gambir Leaf Extract-Modified NiFe LDH Composites: A Study of Cationic Dye Adsorption</dc:title>
	<dc:creator>Jefri, Jefri</dc:creator>
	<dc:creator>Fithri, Najma Annuria</dc:creator>
	<dc:creator>Lesbani, Aldes</dc:creator>
	<dc:subject xml:lang="en-US">NiFe LDH; Uncaria gambir; Malachite Green; Physisorption-Chemisorption; Composite</dc:subject>
	<dc:description xml:lang="en-US">A NiFe layered double hydroxide (LDH) composite with Uncaria gambir (UG) leaf extract was successfully synthesized. The composite (NiFe-UG LDH) and the base material (NiFe LDH) were identified using X-ray Diffraction (XRD), Fourier Transform Infra Red (FTIR), and Brunauer-Emmett-Teller (BET) Surface Area techniques. The XRD and FTIR results revealed the incorporation of gambier leaf extract into the NiFe LDH structure, as indicated by the combined diffraction patterns and spectral features. The BET analysis indicated a decrease in the surface area of NiFe-UG LDH compared to that of NiFe LDH, suggesting that active compounds from the gambier leaf extract effectively coated the LDH surface and blocked its pores. During malachite green (MG) adsorption, NiFe-UG demonstrated faster adsorption kinetics and a higher adsorption efficiency, reaching 96.420% compared to 92.085% for NiFe LDH. While both materials followed pseudo-first-order kinetics, their isotherm behaviors differed: NiFe-UG adhered to the Langmuir model, indicating monolayer adsorption, whereas NiFe LDH followed the Freundlich model, signifying multilayer adsorption. Further analysis suggested that adsorption in NiFe LDH was primarily governed by physisorption, while in NiFe-UG, a combined physisorption-chemisorption mechanism occurred. These results underscore the enhanced adsorption capacity of the composite material, attributed to the introduction of additional functional groups from the gambier leaf extract. Copyright © 2024 by Authors, Published by BCREC Publishing Group. This is an open access article under the CC BY-SA License (https://creativecommons.org/licenses/by-sa/4.0).</dc:description>
	<dc:publisher xml:lang="en-US">Masyarakat Katalis Indonesia - Indonesian Catalyst Society (MKICS)</dc:publisher>
	<dc:date>2024-12-30</dc:date>
	<dc:type>info:eu-repo/semantics/article</dc:type>
	<dc:type>info:eu-repo/semantics/publishedVersion</dc:type>
	<dc:type xml:lang="en-US"></dc:type>
	<dc:format>application/pdf</dc:format>
	<dc:identifier>https://journal.bcrec.id/index.php/bcrec/article/view/20215</dc:identifier>
	<dc:identifier>10.9767/bcrec.20215</dc:identifier>
	<dc:source xml:lang="en-US">Bulletin of Chemical Reaction Engineering &amp; Catalysis; 2024: BCREC Volume 19 Issue 4 Year 2024 (December 2024); 573-584</dc:source>
	<dc:source>1978-2993</dc:source>
	<dc:language>eng</dc:language>
	<dc:relation>https://journal.bcrec.id/index.php/bcrec/article/view/20215/9737</dc:relation>
	<dc:relation>https://journal.bcrec.id/index.php/bcrec/article/downloadSuppFile/20215/5299</dc:relation>
	<dc:relation>https://journal.bcrec.id/index.php/bcrec/article/downloadSuppFile/20215/5300</dc:relation>
	<dc:rights xml:lang="en-US">Copyright (c) 2024 by Authors, Published by BCREC Publishing Group</dc:rights>
	<dc:rights xml:lang="en-US">https://creativecommons.org/licenses/by-sa/4.0</dc:rights>
</oai_dc:dc>