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The Impact of Hydrogen Peroxide as An Oxidant for Solvent-free Liquid Phase Oxidation of Benzyl Alcohol using Au-Pd Supported Carbon and Titanium Catalysts

Bulletin of Chemical Reaction Engineering & Catalysis · Vol. ume (2018) · hlm. 373–385

DOI
10.9767/bcrec.13.2.1204.373-385
ISSN
1978-2993
Terbit
2018-08-01
Penerbit
Masyarakat Katalis Indonesia - Indonesian Catalyst Society (MKICS)
Bahasa
eng
Lisensi
creativecommons.org/licenses/by-sa/4.0

Abstrak

The solvent free oxidation of benzyl alcohol was conducted employing Au and Pd supported catalysts, while utilizing hydrogen peroxide 35% (H2O2) as the oxidant, H2O2 is very cheap, mild, and an environment friendly reagent, which produced water as the only by-product. Various proportions of Au-Pd catalysts on carbon and titanium oxide activated as supports were synthesized through the use of sol immobilization catalyst synthesis technique. Characterization of the synthesized catalysts was performed using X-Ray Diffraction (XRD), Brunauer-Emmett-Teller (BET), Field Emission Scanning Electron Microscopy (FESEM), and Transmission Electron Microscopy (TEM). It was found that the synthesized Au-Pd/ activated carbon catalyst was beneficial for the solvent free oxidation of benzyl alcohol after its containing high surface area measuring 871 m2g-1. Analysis of the TEM data and particle dimension revealed smaller and narrower particle size of 1 wt%. Thus, the distribution of Au-Pd/C was attained. Carbon-supported bimetallic catalysts presented a higher conversion compared to catalysts that are supported titanium oxide (TiO2) for for the oxidation reaction of benzyl alcohol. It was determined that this technique was a suitable process for catalyst synthesis with high selectivity, same distribution of the particle size and activations.

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  • Universitas Syiah Kuala
  • University of Technology Malaysia
  • Chonnam National University
  • State University of Makassar
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Rekan penulisOrganisasiArtikel bersama
Sharifah OsmanAfiliasi tidak diketahui2
Norulhuda IsmailAfiliasi tidak diketahui2
George Tan Geok ShimAfiliasi tidak diketahui2
Bomi ShinChonnam National University1
Cut KhairunnisakUniversitas Syiah Kuala1
Rahmah JoharUniversitas Syiah Kuala1
Cut Morina ZubainurUniversitas Syiah Kuala1
Liza IndriyaniUniversitas Syiah Kuala1
Israa A. JazeelAfiliasi tidak diketahui1
Attared F. HassanAfiliasi tidak diketahui1
Ali AldoghachiAfiliasi tidak diketahui1
Faris A. Jasim Al-DoghachiAfiliasi tidak diketahui1
Surahim MohamadAfiliasi tidak diketahui1
Mukhamad NurhadiAfiliasi tidak diketahui1
Sin Yuan LaiAfiliasi tidak diketahui1
Yubei GuoAfiliasi tidak diketahui1
Chien Yong GohAfiliasi tidak diketahui1
Alysa LauAfiliasi tidak diketahui1
Abdulkareem Ghassan AlsultanAfiliasi tidak diketahui1
Raja Mohamad Hafriz Raja ShahruzzamanAfiliasi tidak diketahui1
Salmiaton AliAfiliasi tidak diketahui1
Robiah YunusAfiliasi tidak diketahui1
Hisyam IhsanAfiliasi tidak diketahui1
Muhammad Ammar NaufalState University of Makassar1
Mohd Salleh AbuAfiliasi tidak diketahui1
Rondiyah RondiyahAfiliasi tidak diketahui1
Nurul ShidaAfiliasi tidak diketahui1
Abdul Hakim Abd JalilAfiliasi tidak diketahui1
Nor Hasniza IbrahimUniversity of Technology Malaysia1
Johari SurifUniversity of Technology Malaysia1
Low Suan EeAfiliasi tidak diketahui1
Corrienna Abdul TalibAfiliasi tidak diketahui1
Mohamad Ikram ZakariaAfiliasi tidak diketahui1
Nik Abdul Hadi Noor NasranAfiliasi tidak diketahui1
Najua Syuhada Ahmad AlhassoraAfiliasi tidak diketahui1

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Sumber metadata: OAI-PMH (metadata jurnal) https://journal.bcrec.id/index.php/bcrec/oai, pertama di-harvest 8 Nov 2026, terakhir terlihat 8 Nov 2026.
Metadata asli (oai_dc) 
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	<dc:title xml:lang="en-US">The Impact of Hydrogen Peroxide as An Oxidant for Solvent-free Liquid Phase Oxidation of Benzyl Alcohol using Au-Pd Supported Carbon and Titanium Catalysts</dc:title>
	<dc:creator>Sanaa Tareq, Sarhan</dc:creator>
	<dc:creator>Saiman, Mohd. Izham</dc:creator>
	<dc:creator>Yun Hin, Taufiq-Yap</dc:creator>
	<dc:creator>Abdullah, Abdul Halim</dc:creator>
	<dc:creator>Rashid, Umer</dc:creator>
	<dc:subject xml:lang="en-US">Benzyl Alcohol; Solvent Free Oxidation; Hydrogen Peroxide; Palladium and Gold Supported Catalyst</dc:subject>
	<dc:description xml:lang="en-US">The solvent free oxidation of benzyl alcohol was conducted employing Au and Pd supported catalysts, while utilizing hydrogen peroxide 35% (H2O2) as the oxidant, H2O2 is  very cheap, mild, and an environment friendly reagent, which produced water as the only by-product. Various proportions of Au-Pd catalysts on carbon and titanium oxide activated as supports were synthesized through the use of sol immobilization catalyst synthesis technique. Characterization of the synthesized catalysts was performed using X-Ray Diffraction (XRD), Brunauer-Emmett-Teller (BET), Field Emission Scanning Electron Microscopy (FESEM), and Transmission Electron Microscopy (TEM). It was found that the synthesized Au-Pd/ activated carbon catalyst was  beneficial for the solvent free oxidation of benzyl alcohol after its containing high surface area measuring 871 m2g-1. Analysis of the TEM data and particle dimension revealed smaller and narrower particle size of 1 wt%. Thus, the distribution of Au-Pd/C was attained. Carbon-supported bimetallic catalysts presented a higher conversion compared to catalysts that are supported titanium oxide (TiO2) for for the oxidation reaction of benzyl alcohol. It was determined that this technique was a suitable process for catalyst synthesis with high selectivity, same distribution of the particle size and activations. </dc:description>
	<dc:publisher xml:lang="en-US">Masyarakat Katalis Indonesia - Indonesian Catalyst Society (MKICS)</dc:publisher>
	<dc:contributor xml:lang="en-US">Universiti Putra Malaysia</dc:contributor>
	<dc:date>2018-08-01</dc:date>
	<dc:type>info:eu-repo/semantics/article</dc:type>
	<dc:type>info:eu-repo/semantics/publishedVersion</dc:type>
	<dc:type xml:lang="en-US"></dc:type>
	<dc:format>application/pdf</dc:format>
	<dc:identifier>https://journal.bcrec.id/index.php/bcrec/article/view/1204</dc:identifier>
	<dc:identifier>10.9767/bcrec.13.2.1204.373-385</dc:identifier>
	<dc:source xml:lang="en-US">Bulletin of Chemical Reaction Engineering &amp; Catalysis; 2018: BCREC Volume 13 Issue 2 Year 2018 (August 2018); 373-385</dc:source>
	<dc:source>1978-2993</dc:source>
	<dc:language>eng</dc:language>
	<dc:relation>https://journal.bcrec.id/index.php/bcrec/article/view/1204/1518</dc:relation>
	<dc:rights xml:lang="en-US">Copyright (c) 2018 by Authors, Published by BCREC Group</dc:rights>
	<dc:rights xml:lang="en-US">http://creativecommons.org/licenses/by-sa/4.0</dc:rights>
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